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  • Palladium-catalyzed carbonylative Heck reaction of aryl bromides with vinyl ethers to 3-alkoxy alkenones and pyrazoles.

Palladium-catalyzed carbonylative Heck reaction of aryl bromides with vinyl ethers to 3-alkoxy alkenones and pyrazoles.

Chemistry (Weinheim an der Bergstrasse, Germany) (2012-03-17)
Johannes Schranck, Xiao-Feng Wu, Helfried Neumann, Matthias Beller
초록

Three COming together: The first carbonylative Heck coupling reaction of aryl bromides and vinyl ethers leading to 1-aryl-3-alkoxy-2-propen-1-ones has been established (see scheme). Based on this coupling methodology, a novel one-pot synthesis of aryl-substituted pyrazoles was also realized.

MATERIALS
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Sigma-Aldrich
Palladium(II) bromide, 99%